Analysis of halogenated flame retardants in Canadian wastewater treatment plants using gas chromatography–tandem mass spectrometry (GC-MS/MS)

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dc.contributor.author
Shanmuganathan, Meera
Zhang, Zifeng
Sverko, Ed
Brymer, Rachel
Gill, Biban
Smyth, Shirley Anne
dc.date.accepted
2018-07-03
dc.date.accessioned
2024-01-23T20:45:30Z
dc.date.available
2024-01-23T20:45:30Z
dc.date.issued
2018-11-01
dc.date.submitted
2017-10-30
dc.description.abstract - en
An investigation of brominated flame retardants (BFRs), polybrominated diphenylethers (PBDEs), and chlorinated flame retardants was conducted in samples from Canadian wastewater treatment plants (WWTPs). The penta-BDE mixture and deca-BDE were most commonly detected. Median removal efficiencies of PBDEs by WWTPs were 71% to 99% and higher concentrations of PBDEs were found in influent samples in summer, compared to winter. Three novel brominated flame retardants (nBFRs) including 1,2-bis(2,4,6-tribromophenoxy)ethane (BTBPE), 2-ethylhexyl-2,3,4,5-tetrabromobenzoate (EHTeBB or TBB), and bis(2-ethyl-1-hexyl)tetrabromophthalate (BEHTBP or TBPH) were detected in greater than 80% of influents and biosolids. Median removal efficiencies were 45% to 99% for BTBPE, 63% to 99% for TBB, and 88% to 99% for TBPH. Detection of total dechlorane plus ((DP) syn and anti) was greater than 90% in both wastewater and biosolids samples. However, median removal efficiencies were between 51% and 66% for total DP. Overall, PBDEs were effectively removed via different treatment processes, while BTBPE, TBB, and DP exhibited lower removal rates, which could be due to their physical chemical properties.
dc.identifier.doi
https://doi.org/10.2166/wqrj.2018.040
dc.identifier.issn
2709-8052
2709-8044
dc.identifier.uri
https://open-science.canada.ca/handle/123456789/1887
dc.language.iso
en
dc.publisher
IWA Publishing
dc.rights - en
Creative Commons Attribution 4.0 International (CC BY 4.0)
dc.rights - fr
Creative Commons Attribution 4.0 International (CC BY 4.0)
dc.rights.openaccesslevel - en
Gold
dc.rights.openaccesslevel - fr
Or
dc.rights.uri - en
https://creativecommons.org/licenses/by/4.0/
dc.rights.uri - fr
https://creativecommons.org/licenses/by/4.0/deed.fr
dc.subject - en
Nature and environment
Water
Science and technology
dc.subject - fr
Nature et environnement
Eau
Sciences et technologie
dc.subject.en - en
Nature and environment
Water
Science and technology
dc.subject.fr - fr
Nature et environnement
Eau
Sciences et technologie
dc.title - en
Analysis of halogenated flame retardants in Canadian wastewater treatment plants using gas chromatography–tandem mass spectrometry (GC-MS/MS)
dc.type - en
Article
dc.type - fr
Article
local.article.journalissue
4
local.article.journaltitle
Water Quality Research Journal
local.article.journalvolume
53
local.pagination
167–180
local.peerreview - en
Yes
local.peerreview - fr
Oui
local.requestdoi
No
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